间歇反应与精馏强化过程的二维实时优化与动态协同控制研究

项目来源

国家自然科学基金(NSFC)

项目主持人

薄翠梅

项目受资助机构

南京工业大学

立项年度

2016

立项时间

未公开

项目编号

61673205

项目级别

国家级

研究期限

未知 / 未知

受资助金额

62.00万元

学科

信息科学-自动化-控制系统与应用

学科代码

F-F03-F0302

基金类别

面上项目

关键词

协调控制 ; 间歇反应精馏过程 ; 控制结构设计 ; 动态优化 ; 二维系统 ; Batch Reaction Distillation ; two-dimension system ; Dynamic Optimization ; Cooperative Control ; Design of control structure

参与者

汤吉海;李丽娟;杨世品;易辉;黄庆庆;黄燕;牛超;郭伟;杨磊

参与机构

南京工业大学

项目标书摘要:间歇反应与精馏强化技术,通过反应能力与分离能力相互协同作用,可有效提高资源/能源利用率,减少污染。课题根据间歇反应精馏过程多时序、强耦合、非线性特性,研究基于两维(批次+时间)动态信息的实时优化操作与动态协同控制方法,拟解决废液循环利用的批间优化操作与生产调度问题。内容如下:1)建立间歇反应精馏动态数学模型,研究强化过程物料转化与能量利用机制,设计经济集成优化算法获取反应与分离能力最佳匹配的集成结构。2)研究基于经济模型的动态优化与控制协同算法,实现最佳操作轨迹、最短生产周期与跟踪控制同步优化;研究基于批次容量最大化的批间优化控制算法,实现废液批间循环的可持续操作。3)研究二维多模型广义预测迭代控制算法,实现不确定条件下的快速跟踪控制。4)以理想四元可逆反应体系体系为例,研制间歇反应精馏过程一体化流程模拟系统。课题研究对发挥反应精馏过程的高转化率、高选择性、低能耗集成优势具有重要意义。

Application Abstract: The batch reaction and distillation reinforcement technology can improve the utilization of resources and energy,and reduce the pollution by the interaction of reaction and separation capacity.Based on the complex characteristics of batch reactive distillation processes such as multi-time series,strong coupling and nonlinearity,the dynamic optimization and cooperative control methods based on two dimensional(Batch+Time)dynamic information will be studied in the project in order to solve the optimized operation and scheduling problems between batch-to-batch waste-liquor recycling.The following items will be discussed:1)The dynamic mechanism model will be established based on material conversion and energy utilization mechanism,and the optimal matching condition of reaction and separation capacity will be achieved by the economic integration optimization algorithm.2)Algorithm of batch simultaneous model-based optimization and control(BSMBOC)will be researched to obtain optimal operation trajectory and the shortest batch time.And the optimization method based on maximizing batch capacity will be researched to realize the sustainable operation with batch-to-batch waste-liquor recycling.3)The multi-model generalized predictive iterative learning control algorithm(MGPILC)based on two dimensional system will be researched for efficient and accurate tracking control under the uncertain condition.4)An all-in-one simulation experiment system will be built based on the ideal quaternary reversible reaction system.This subject will benefit to developing the integration advantages,such as the high conversion rate,high selectivity and low energy consumption of the reactive distillation processes.

项目受资助省

江苏省

项目结题报告(全文)

间歇反应精馏强化技术,通过反应与分离能力相互协同作用,可有效提高资源和能源利用率,减少和预防污染。本课题根据间歇反应精馏过程多时序、强耦合、周期性特性,利用二维(批次+时间)动态信息,研究了不确定条件下过程实时优化与动态协同控制方法,选取理想的四元可逆反应体系、醋酸甲酯反应体系为例,研制多批次间歇反应精馏过程一体化流程模拟实验系统,验证上述算法的有效性。该项目取得的研究成果目前已累积发表学术论文32篇(其中SC1收录10篇,EIISTP收录18篇),申请国家技术发明专利7项,其中已授权1项,已受理公开6项,培养研究生11名,毕业硕士研究生8名。主要研究内容和结果有:(1)建立了反应精馏过程动态数学模型及提出了快速求解方法;利用非支配遗传算法获取间歇反应精馏过程的最佳集成结构和操作参数,在对强化过程物料转化与能量利用机制研究基础上,通过经济集成优化算法实现反应能力与分离能力的最佳匹配设计;(2)提出基于经济模型的实时优化和动态协同控制算法(BSMBOC算法),通过经济指标与批间最大循环周期数建立综合优化目标函数,将关键变量操作轨迹、最短操作时间与底层跟踪控制同步优化计算,不断优化操纵变量和操作时间的轨迹,以及更新关键操纵变量的控制区域与控制周期,实现废液批间循环的可持续操作。(3)在二维系统迭代学习的基础上,建立了全周期的二维等效过程模型(2D-CARIMA);分别研究了二维PID迭代学习控制算法(2D-PIDILC)和二维广义预测迭代学习控制算法(2D-MGPILC);(4)选取理想的四元可逆反应体系和醋酸甲酯反应体系为例,分别进行批内过程优化算法、基于废液循环的批间优化算法、2D-MGPILC算法的模拟实验验证研究,使用ASPEN PLUS、MATLAB、SupOS平台,研制多批次间歇反应精馏过程一体化流程模拟实验系统,验证上述算法的有效性。上述研究结果,可为实际工程设计提供理论依据,对于丰富间歇过程的协同控制理论内容,以及发挥反应精馏过程高转化率、高选择性、低能耗集成优势具有重要意义与参考价值。

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  • 1.A Dynamic Feature Regression Network for Industrial Soft Sensor Modeling

    • 关键词:
    • Carbon monoxide;Convolutional neural networks;Ethylene;Ethylene glycol;Extraction;Long short-term memory;Quality control;Regression analysis;Supervised learning;Auto encoders;Autoencoder network;Convolutional neural network;Dynamic features;Features extraction;Long short-term memory network;Memory network;Semi-supervised learning;Soft sensors
    • Yang, Cheng;Gao, Shida;Jiang, Chao;Zhang, Quanlin;Li, Jun;Bo, Cuimei
    • 《42nd Chinese Control Conference, CCC 2023》
    • 2023年
    • July 24, 2023 - July 26, 2023
    • Tianjin, China
    • 会议

    Soft sensor has been extensively applied for online estimation of the key quality variables in modern industrial processes, which is extremely important for the process to achieve efficient monitoring and smooth control. To build an accurate data-driven model, the dynamic correlation and strong nonlinearity of process sequential data must be considered in soft sensor modeling. Therefore, a dynamic feature regression network (DFR) is proposed in this paper for industrial soft sensor modeling, consisting of a dynamic feature extraction network and a feature regression network to explore different industrial data features. First, the dynamic feature extraction network maps time series samples to a set of hidden dynamic features, while the feature regression network performs deeper feature extraction and output regression on key quality variables. Furthermore, since both networks consist of unsupervised feature extraction and supervised feature regression, a large scale of unlabeled samples can be utilized in the semisupervised learning of model parameters. Finally, the feasibility and efficacy of the proposed model are verified through the coal-to-ethylene glycol process data to predict the carbon monoxide content. © 2023 Technical Committee on Control Theory, Chinese Association of Automation.

    ...
  • 2.多批次间歇反应过程的二维迭代学习PI控制方法

    • 关键词:
    • 间歇反应;二维系统;迭代学习
    • 杨磊;李想;薄翠梅;张广明
    • 《第28届中国过程控制会议(CPCC 2017)暨纪念中国过程控制会议30周年》
    • 中国重庆
    • 会议

    本文针对工业过程中最常用的间歇补料反应过程,利用间歇过程的重复性和二维动态特性,以二维系统理论为基础,二维系统的状态空间模型,分析迭代学习控制的二维特性。将传统的PI控制器作为内环结构,使用迭代学习控制器优化其参考轨迹,得到基于二维系统的迭代学习PI控制方法(ILC-PI方法),并通过稳定性分析确定控制器参数选择方式。将ILC-PI控制方法应用于一类多批次间歇补料反应过程中,结果表明,虽然初始收敛速率较低,但是随着批次不断优化,最终的跟踪性能较好。

    ...
  • 3.COORDINATED SYNCHRONIZATION CONTROL OF MULTI-MOTOR SYSTEM BASED ON SYNERGETIC CONTROL THEORY

    • 《第30届中国控制与决策会议》
    • 2018-06-09
    • 中国辽宁沈阳
    • 会议

    A synergetic speed controller(SSC) is proposed for the multi-motor system of triple brushless DC(BLDC) motors with the relative coupling structure in order to improve the coordination and robustness.To achieve the desired synchronous control objective,an augmented dynamic model of the BLDC motor is firstly developed.Based on the synergetic control theory,a manifold is then constructed for the ith motor as the linear combination of the phase current,the speed tracking error and its integration,and the coordination error as well as its integration.The control law of the SSC is further deduced from the augmented model and the manifold.The effects of controller parameters on the synchronization performance and their selection principle are also discussed.Simulative results on the triple-BLDC motor system with relative coupling show that the SSC can provide better synchronization and robustness,by comparing with the conventional PID relative coupling control and the sliding mode control(SMC) relative coupling control.

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  • 4.Dynamic Control Allocation Fault-Tolerant Method for a Class of Distributed Control Systems

    • 关键词:
    • Robust control ; Fault tolerance ; Linear matrix inequalities ; Real time systems ; Distributed parameter control systems ; Constrained optimization ; State space methods;Augmented state space ; Co;operative control ; Control allocation ; Dynamic control allocations ; Fault tolerant control ; Fault;tolerant method ; Hierarchical structures ; Leveling control systems
    • ZhangShenpeng;ZhangDengfeng;ZhangZhaodong;ZhangQi;LuBaochun
    • 《37th Chinese Control Conference, CCC 2018》
    • 2018年
    • July 25, 2018 - July 27, 2018
    • Wuhan, China
    • 会议

    The dynamic control allocation algorithm is proposed for a class of distributed control systems with hierarchical structure, in order to solve the real-time cooperative control problem in the case of sensor failure occurred in the subsystems. The augmented state-space model of the distributed control system is first established for the control allocation design, by using the dynamic model of sensor faults. According to robust control theory, the constrained and convex optimization is then formulated into linear-matrix-inequality form to design the gain matrix of the control allotter, which can be computed by various well-developed algorithms. Thus the suppression of sensor faults in the subsystem is realized and the expected cooperative control objective is achieved. Simulations on the four-corner leveling control system of an advanced hydraulic press demonstrate the effectiveness of the proposed control allocation algorithm. © 2018 Technical Committee on Control Theory, Chinese Association of Automation.

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  • 5.Dynamic Control Design and Simulation of Biogas Pressurized Water Scrubbing Process

    • 关键词:
    • Biogas; pressurized water scrubbing; optimal design; plant level dynamiccontrol; Aspen plus
    • Bo Cuimei;Guo Wei;Tang Chao;Li Jun;Lu Xiaohua
    • 《10th IFAC Symposium on Advanced Control of Chemical Processes 》
    • 2018年
    • JUL 25-27, 2018
    • Shenyang, PEOPLES R CHINA
    • 会议

    For the process of biogas pressurized water scrubbing, design and simulation of plant-level dynamic control system is researched based on the optimum structure and parameters of the steady state in this paper. According to the process requirements of the biogas pressurized water scrubbing pilot-scale plant, a steady state simulation system is established using Aspen Plus. The simulation research under different operation conditions is carried out to obtain the optimal operating parameters. Then plant-level dynamic control schemes and the dynamic simulation system are also designed to ensure the efficiency of biogas purification. The system's performance is tested under introducing biogas inlet flow disturbance and intake flow component disturbance. The simulation results show that the system has good dynamic response performance, such as the removal rate of CO2 is greater than 99.8% under various disturbances. (C) 2018, IFAC (International Federation of Automatic Control) Hosting by Elsevier Ltd. All rights reserved.

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  • 6.Multi-objective Optimization of Methyl Acetate Hydrolysis Process Based on NSGA-ⅡAlgorithm

    • 《第30届中国控制与决策会议》
    • 2018-06-09
    • 中国辽宁沈阳
    • 会议

    An enhanced non-dominated sorting genetic algorithm(NSGA-II) was applied to carry out the integer optimized design in this article.The steady simulation design was established based on the reaction kinetics analysis using Aspen Plus,and the feasible region of each optimized variable was calculated through sensitive analysis.Aiming at the total cost TAC as the objective function,the NSGA-II algorithm was used directly to obtain the Pareto optimal solutions under the constraints of feasible region of variables.The simulation results showed that the NSGA-II algorithm can effectively reduce the total cost of TAC.

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  • 7.基于NSGA-Ⅱ算法的醋酸甲酯水解工艺过程多变量优化方法

    • 关键词:
    • NSGA-Ⅱ算法;多变量优化;稳态模拟;醋酸甲酯水解
    • 薄翠梅;郭伟;尹俊华;黄燕;李俊
    • 《第28届中国过程控制会议(CPCC 2017)暨纪念中国过程控制会议30周年》
    • 中国重庆
    • 会议

    本文针对醋酸甲酯水解生产工艺优化设计问题,采用改进的非支配遗传算法(NSGA-II算法)开展厂级多变量经济优化设计。在反应动力学分析基础上进行Aspen Plus稳态模拟设计,通过灵敏分析计算出每个优化变量的可行域;以年总成本TAC为优化目标函数、优化变量可行域为约束,运用非支配遗传算法NSGA-II直接对Aspen Plus中反应精馏塔和甲醇回收塔的稳态模型进行多变量优化计算,将优化结果和序贯优化结果相比较,NSGA-II多变量同步优化算法更易寻找到全局最优解,大大降低了生产总投资成本。

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  • 8.多批次间歇反应过程的二维迭代学习PI控制方法

    • 关键词:
    • 间歇反应;二维系统;迭代学习
    • 杨磊;李想;薄翠梅;张广明
    • 《第28届中国过程控制会议(CPCC 2017)暨纪念中国过程控制会议30周年》
    • 中国重庆
    • 会议

    本文针对工业过程中最常用的间歇补料反应过程,利用间歇过程的重复性和二维动态特性,以二维系统理论为基础,二维系统的状态空间模型,分析迭代学习控制的二维特性。将传统的PI控制器作为内环结构,使用迭代学习控制器优化其参考轨迹,得到基于二维系统的迭代学习PI控制方法(ILC-PI方法),并通过稳定性分析确定控制器参数选择方式。将ILC-PI控制方法应用于一类多批次间歇补料反应过程中,结果表明,虽然初始收敛速率较低,但是随着批次不断优化,最终的跟踪性能较好。

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